- Emma Thompson Character (Nanny McPhee)
- Colin Firth Character (Mr. Brown)
- Kelly Macdonald Character (Evangeline)
- Thomas Sangster Character (Simon)
- Eliza Bennett Character (Tora)
- Raphal Coleman Character (Eric)
- Samuel Honywood Character (Sebastian)
- Angela Lansbury Character (Aunt Adelaide)
- Celia Imrie Character (Mrs. Quickly)
- Imelda Staunton Character (Mrs. Blatherwick)
- Elizabeth Berrington Character (Letita)
- Derek Jacobi Character (Mr. Wheen)
- Phyllida Law Character (Mrs. Partridge (voice))
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